Litcius/Paper detail

Cd<sup>2+</sup> Detection by an Electrochemical Electrode Based on MWCNT–Orange Peel Activated Carbon

Luis C. Beas-Bernuy, Andy A. Cardenas‐Riojas, Sandy L. Calderon‐Zavaleta, Ulises Quiroz‐Aguinaga, Adolfo La Rosa-Toro, Elvis O. López, Yvan Jesús Olortiga Asencios, Angélica M. Baena‐Moncada, Golfer Muedas‐Taipe

2023ACS Omega22 citationsDOIOpen Access PDF

Abstract

High Resolution Image Download MS PowerPoint Slide This study reports the development of a new electrochemical sensor based on a carbon paste electrode (CPE) composed of biomass-based orange peel activated carbon (ACOP) and multiwalled carbon nanotubes (MWCNTs), and this composite is used for the electrochemical detection of cadmium ions (Cd 2+ ). The ACOP/MWCNT composite was characterized by FTIR, Raman, and electrochemical impedance spectroscopy. The electrochemical evaluation of Cd 2+ was performed using square wave and cyclic voltammetry. The ACOP/MWCNT–CPE electrochemical sensor exhibited a coefficient of determination r 2 of 0.9907, a limit of detection of 0.91 ± 0.79 μmol L –1, and a limit of quantification of 3.00 ± 2.60 μmol L –1 . In addition, the developed sensor can selectively detect Cd 2+ in the presence of different interferents such as Zn 2+, Pb 2+, Ni 2+, Co 2+, Cu 2+, and Fe 2+ with a relative standard deviation (RSD) close to 100%, carried out in triplicate experiments. The ACOP/MWCNT–CPE presented high sensitivity, stability, and reproducibility and was successfully applied for the detection of Cd 2+ in river water samples with recovery rate values ranging from 97.33 to 115.6%, demonstrating to be a very promising analytical alternative for the determination of cadmium ions in this matrix.

Topics & Concepts

Detection limitAnalytical Chemistry (journal)ElectrochemistryMaterials scienceElectrochemical gas sensorCyclic voltammetryCarbon nanotubeRaman spectroscopyNuclear chemistryElectrodeDielectric spectroscopyCadmiumMetal ions in aqueous solutionChemistryMetalNanotechnologyChromatographyPhysical chemistryMetallurgyOpticsPhysicsElectrochemical Analysis and ApplicationsElectrochemical sensors and biosensorsConducting polymers and applications