Litcius/Paper detail

CuO@In<sub>2</sub>O<sub>3</sub>/ZnO Core–Shell Nanorods for Triethylamine Detection at Room Temperature

Baoye Zi, Mingpeng Chen, Qin Zhu, Qingjie Lu, Bin Xiao, Zongming Deng, Dong Xu, Zhenlin Song, Jianhong Zhao, Yumin Zhang, Zhongqi Zhu, Jin Zhang, Qingju Liu

2023ACS Applied Nano Materials23 citationsDOI

Abstract

Sensitive and stable triethylamine (TEA) gas sensors are desirable for environmental and human safety. However, the high operating temperature of the metal-oxide-based gas sensors poses a limitation on their wide applications. Herein, we fabricate an exceptional TEA gas sensor based on the core–shell heterostructure comprising crystalline CuO and amorphous In 2 O 3 /ZnO (CuInZnO) via a facile electrodeposition method. Remarkably, the optimum gas sensor (CuInZnO-3) exhibits an outstanding gas response (∼25) toward a 10 ppm TEA at room temperature. Moreover, CuInZnO-3 shows excellent selectivity, linear response, and stability. The superior sensing performance can be mainly ascribed to the unique core–shell nanorod heterostructure with a high specific surface area, allowing the formation of p–n junctions. The amorphous nature of the In 2 O 3 /ZnO shell also enriches the active oxygen on the surface and enhances gas adsorption.

Topics & Concepts

NanorodAmorphous solidHeterojunctionMaterials scienceTriethylamineAdsorptionShell (structure)OxideNanotechnologySelectivityChemical engineeringOptoelectronicsCatalysisChemistryPhysical chemistryComposite materialCrystallographyMetallurgyOrganic chemistryBiochemistryEngineeringGas Sensing Nanomaterials and SensorsAdvanced Chemical Sensor TechnologiesAnalytical Chemistry and Sensors