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Imaging orbital ferromagnetism in a moiré Chern insulator

C. L. Tschirhart, M. Serlin, H. Polshyn, A. Shragai, Z. Xia, J. Zhu, Y. Zhang, K. Watanabe, T. Taniguchi, M. E. Huber, A. F. Young

2021Science196 citationsDOIOpen Access PDF

Abstract

Electrons in moiré flat band systems can spontaneously break time-reversal symmetry, giving rise to a quantized anomalous Hall effect. In this study, we use a superconducting quantum interference device to image stray magnetic fields in twisted bilayer graphene aligned to hexagonal boron nitride. We find a magnetization of several Bohr magnetons per charge carrier, demonstrating that the magnetism is primarily orbital in nature. Our measurements reveal a large change in the magnetization as the chemical potential is swept across the quantum anomalous Hall gap, consistent with the expected contribution of chiral edge states to the magnetization of an orbital Chern insulator. Mapping the spatial evolution of field-driven magnetic reversal, we find a series of reproducible micrometer-scale domains pinned to structural disorder.

Topics & Concepts

Condensed matter physicsMagnetizationPhysicsMagnetismQuantum anomalous Hall effectBilayer grapheneOrbital magnetizationQuantum Hall effectFerromagnetismSuperconductivityElectronInsulator (electricity)Bohr modelSpontaneous magnetizationMagnetic fieldQuantumMagnetic domainHall effectCharge (physics)GrapheneBilayerTopological insulatorGraphene research and applicationsTopological Materials and PhenomenaChemical and Physical Properties of Materials