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Enhanced triplet superconductivity in next-generation ultraclean UTe <sub>2</sub>

Z. Wu, Theodore I. Weinberger, Jiasheng Chen, A. Cabala, Dmitry V. Chichinadze, Daniel J. Shaffer, Jiří Pospíšil, Ján Prokleška, Tetiana Haidamak, Gaël Bastien, V. Sechovský, A. J. Hickey, M. J. Mancera-Ugarte, Shermane M. Benjamin, David Graf, Y. Skourski, G. G. Lonzarich, Michal Vališka, F. M. Grosche, Alexander G. Eaton

2024Proceedings of the National Academy of Sciences30 citationsDOIOpen Access PDF

Abstract

The unconventional superconductor UTe[Formula: see text] exhibits numerous signatures of spin-triplet superconductivity-a rare state of matter which could enable quantum computation protected against decoherence. UTe[Formula: see text] possesses a complex phase landscape comprising two magnetic field-induced superconducting phases, a metamagnetic transition to a field-polarized state, along with pair- and charge-density wave orders. However, contradictory reports between studies performed on UTe[Formula: see text] specimens of varying quality have severely impeded theoretical efforts to understand the microscopic origins of the exotic superconductivity. Here, we report a comprehensive suite of high magnetic field measurements on a generation of pristine quality UTe[Formula: see text] crystals. Our experiments reveal a significantly revised high magnetic field superconducting phase diagram in the ultraclean limit, showing a pronounced sensitivity of field-induced superconductivity to the presence of crystalline disorder. We employ a Ginzburg-Landau model that excellently captures this acute dependence on sample quality. Our results suggest that in close proximity to a field-induced metamagnetic transition the enhanced role of magnetic fluctuations-that are strongly suppressed by disorder-is likely responsible for tuning UTe[Formula: see text] between two distinct spin-triplet superconducting phases.

Topics & Concepts

SuperconductivityAlgorithmField (mathematics)PhysicsPhase diagramCondensed matter physicsPhase (matter)DatabaseTopology (electrical circuits)Materials scienceComputer scienceQuantum mechanicsElectrical engineeringMathematicsEngineeringPure mathematicsRare-earth and actinide compoundsIron-based superconductors researchAdvanced Condensed Matter Physics