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Origin of the unique thermoelectric transport in Mg<sub>3</sub>(Sb,Bi)<sub>2</sub>: absence of d-orbital bonding in crystal cohesion

Ruoyu Wang, Zhe Guo, Qiang Zhang, Jianfeng Cai, Guoqiang Liu, Xiaojian Tan, Jun Jiang

2022Journal of Materials Chemistry A11 citationsDOI

Abstract

Owing to the small periodic number of Mg, the absence of d-orbital bonding is responsible for Mg 3 (Sb,Bi) 2 's unique conduction band dispersion and extraordinarily low lattice thermal conductivity.

Topics & Concepts

Condensed matter physicsThermoelectric effectThermal conductionMaterials scienceConduction bandCohesion (chemistry)Crystal structureThermal conductivityLattice (music)CrystallographyThermoelectric materialsChemistryPhysicsElectronThermodynamicsComposite materialQuantum mechanicsAcousticsAdvanced Thermoelectric Materials and DevicesHeusler alloys: electronic and magnetic propertiesThermal properties of materials
Origin of the unique thermoelectric transport in Mg<sub>3</sub>(Sb,Bi)<sub>2</sub>: absence of d-orbital bonding in crystal cohesion | Litcius