Litcius/Paper detail

High-speed imaging reveals the dynamics of the initiation and subsequent evolution of a nanosecond discharge propagating along the air–water interface

Petr Hoffer, V. Prukner, Garima Arora, Milan Šimek

2023Plasma Sources Science and Technology11 citationsDOIOpen Access PDF

Abstract

Abstract A nanosecond DBD-like discharge in a coplanar electrode configuration propagating along the water–air interface is an efficient source of reactive species to produce plasma-activated water. In this letter, we report on the mechanism of the discharge onset as well as on further developments over hundreds of nanoseconds. We combined ultrafast optical imaging with electrical characteristics to capture basic morphological imprints of individual discharge phases occurring during a single discharge event with high temporal resolution. We show that during the first nanoseconds, a diffuse bi-directional ionizing avalanche expands over the liquid surface at high speed (&gt;5 <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:mo>×</mml:mo> </mml:math> 10 5 m s −1 ). Later, discrete plasma filaments form from the diffuse plasma due to an ionization instability. The filaments, during their subsequent elongation (∼2 <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:mo>×</mml:mo> </mml:math> 10 5 m s −1 ), retain the diffuse plasma at both ends. The filaments re-ignite in the same positions on the liquid surface over several successive (mainly capacitive) current pulses (∼1 μ s apart), which result from discontinuities in the driving voltage.

Topics & Concepts

NanosecondPlasmaIonizationStreamer dischargeAnalytical Chemistry (journal)Classification of discontinuitiesMaterials scienceAtomic physicsPhysicsChemistryOpticsIonLaserMathematical analysisChromatographyQuantum mechanicsMathematicsElectrohydrodynamics and Fluid DynamicsPlasma Applications and DiagnosticsPlasma Diagnostics and Applications