Litcius/Paper detail

Enantioselective Double Carbonylation Enabled by High-Valent Palladium Catalysis

Jian Han, Bo-Wen Xiao, Tian‐Yu Sun, Min Wang, Long Jin, Wangzhi Yu, Yuqin Wang, Dongmei Fang, Yan Zhou, Xiao‐Feng Wu, Yun‐Dong Wu, Jian Liao

2022Journal of the American Chemical Society51 citationsDOI

Abstract

Palladium-catalyzed carbonylation reactions are efficient methods for synthesizing valuable molecules. However, realizing a carbonylation with excellent yield and chemo-, regio-, and enantioselectivities by classical low-valent palladium catalysis is highly challenging. Herein, we describe an enantioselective carbonylation reaction using a high-valent palladium catalysis strategy and employing a chiral sulfoxide phosphine (SOP) ligand. This double aminocarbonylation reaction begins with the formation of a carbamoylpalladium(II) species, which undergoes enantioselective oxidative addition with a cyclic diaryliodonium salt to generate a palladium(IV) intermediate, followed by a second CO insertion and reductive elimination. The mechanism has been illustrated with experimental and computational studies.

Topics & Concepts

ChemistryCarbonylationPalladiumEnantioselective synthesisCatalysisReductive eliminationSulfoxideOxidative additionPhosphineCombinatorial chemistryLigand (biochemistry)Organic chemistryCarbon monoxideBiochemistryReceptorCatalytic C–H Functionalization MethodsCatalytic Cross-Coupling ReactionsAsymmetric Hydrogenation and Catalysis