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Enzyme immobilization strategies for the design of robust and efficient biocatalysts

José M. Guisán, Gloria Fernández‐Lorente, Javier Rocha‐Martín, Daniel Moreno-Gamero

2022Current Opinion in Green and Sustainable Chemistry137 citationsDOIOpen Access PDF

Abstract

Different strategies for the preparation of efficient and robust immobilized biocatalysts are here reviewed. Different physico-chemical approaches are discussed. i.- The stabilization of enzyme by any kind of immobilization on pre-existing porous supports. ii.- The stabilization of enzymes by multipoint covalent attachment on support surfaces. iii.- Additional stabilization of immobilized-stabilized enzyme by physical or chemical modification with polymers. These three strategies can be easily developed when enzymes are immobilized in pre-existing porous supports. In addition to that, these immobilized-stabilized derivatives are optimal to develop enzyme reaction engineering and reactor engineering. Stabilizations ranging between 1000 and 100,000 folds regarding diluted soluble enzymes are here reported.

Topics & Concepts

Immobilized enzymeEnzymeCovalent bondPorosityChemistryPolymerChemical engineeringChemical modificationMaterials scienceCombinatorial chemistryOrganic chemistryPolymer chemistryEngineeringEnzyme Catalysis and ImmobilizationElectrochemical sensors and biosensorsMicrobial Metabolic Engineering and Bioproduction
Enzyme immobilization strategies for the design of robust and efficient biocatalysts | Litcius