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Hydrogen release from liquid organic hydrogen carriers catalysed by platinum on rutile-anatase structured titania

Päivi Aakko-Saksa, Marko Vehkamäki, Marianna Kemell, Laura Keskiväli, Pekka Simell, Matti Reinikainen, Unto Tapper, Timo Repo

2020Chemical Communications53 citationsDOIOpen Access PDF

Abstract

A liquid organic hydrogen carrier (LOHC) is an interesting concept for hydrogen storage. We describe herein a new, active catalyst system for dehydrogenation of perhydrogenated dibenzyl toluene (H18-DBT), which is a promising LOHC candidate. Pt supported on a rutile-anatase form of titania was found to be more active than Pt supported on anatase-only titania, or on alumina, and almost equally active as Pt supported on carbon. Robust and durable metal oxide supports are preferred for catalysing reactions at high temperatures.

Topics & Concepts

DehydrogenationAnataseRutileHydrogenCatalysisPlatinumTolueneHydrogen storageInorganic chemistryMaterials scienceChemistryChemical engineeringPhotochemistryOrganic chemistryPhotocatalysisEngineeringHybrid Renewable Energy SystemsHydrogen Storage and MaterialsAdvanced Battery Materials and Technologies
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