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N, S co-doped porous graphene-like carbon synthesized by a facile coal tar pitch-blowing strategy for high-performance supercapacitors

Gang Li, Shanshan Chen, Yonggang Wang, Gang Wang, Yuhan Wu, Yang Xu

2023Chemical Physics Letters19 citationsDOIOpen Access PDF

Abstract

Herein, coal tar pitch (CTP) derived nitrogen and sulfur co-doped porous graphene-like carbon (NSPC) is performed by an ammonium sulfate-assisted chemical blowing strategy. Afterward, NSPC was activated by KOH to form a-NSPC features a bubble-like structure with a thin porous shell and a well-balanced porous ratio. Serving as electrode materials for supercapacitors, the capacitance of a-NSPC was 368 F g-1 at 0.5 A g-1. Meanwhile, the prepared materials exhibit excellent cycling stability after 10000 cycles. This work may not only prepare superior electrode materials but also provide a feasible strategy for large-scale production of high-performance and low-cost electrode materials.

Topics & Concepts

SupercapacitorMaterials scienceCoal tarCapacitanceChemical engineeringElectrodePorosityCarbon fibersGrapheneSulfurNanotechnologyComposite materialCoalOrganic chemistryChemistryEngineeringComposite numberPhysical chemistryMetallurgySupercapacitor Materials and FabricationAdvancements in Battery MaterialsElectrocatalysts for Energy Conversion