Litcius/Paper detail

Transparent ultrahigh-molecular-weight polyethylene/MXene films with efficient UV-absorption for thermal management

Xianhu Liu, Wenrui Zhang, Xin Zhang, Zhengui Zhou, Chunfeng Wang, Yamin Pan, Bin Hu, Chuntai Liu, Caofeng Pan, Changyu Shen

2024Nature Communications106 citationsDOIOpen Access PDF

Abstract

Abstract The rational use and conversion of energy are the primary means for achieving the goal of carbon neutrality. MXenes can be used for photothermal conversion, but their opaque appearance limits wider applications. Herein, we successfully develop visible-light transparent and UV-absorbing polymer composite film by solution blending the MXene with polyethylene and then vacuum pressing. The resulting film could be quickly heated to 65 °C under 400 mW cm −2 light irradiation and maintained over 85% visible-light transmittance as well as low haze (<12%). The findings of the indoor heat insulation test demonstrate that the temperature of the glass house model covered by this film was 6-7 °C lower than that of the uncovered model, revealing the potential of transparent film in energy-saving applications. In order to mimic the energy-saving condition of the building in various climates, a typical building model with this film as the outer layer of the window was created using the EnergyPlus building energy consumption software. According to predictions, they could reduce yearly refrigeration energy used by 31-61 MJ m −2 , and 3%-12% of the total energy used for refrigeration in such structures. This work imply that the film has wide potential for use as transparent devices in energy-related applications.

Topics & Concepts

OpacityMaterials sciencePhotothermal therapyMXenesAbsorption (acoustics)PolyethylenePolymerCarbon fibersOptoelectronicsThermalNanotechnologyComposite numberChemical engineeringOpticsComposite materialMeteorologyEngineeringPhysicsMXene and MAX Phase MaterialsAdvanced Sensor and Energy Harvesting MaterialsAdvanced Photocatalysis Techniques