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Ni-Catalyzed Denitrogenative Cross-Coupling of Benzotriazinones and Cyclopropanols: An Easy Access to Functionalized β-Aryl Ketones

Jincan Li, Yan Zheng, Mingxian Huang, Wanfang Li

2020Organic Letters64 citationsDOI

Abstract

A novel Ni-catalyzed denitrogenative cross-coupling between benzotriazinones and cyclopropanols is reported herein. This neoteric reactivity allows for the convenient synthesis of β-(o-amido)aryl ketones from readily available starting materials with good yields (up to 93%) and general substrate scope.

Topics & Concepts

ChemistryArylCatalysisScope (computer science)Substrate (aquarium)Reactivity (psychology)Coupling (piping)Combinatorial chemistryCoupling reactionOrganic chemistryComputer sciencePathologyProgramming languageMechanical engineeringEngineeringMedicineGeologyAlternative medicineOceanographyAlkylCatalytic C–H Functionalization MethodsCyclopropane Reaction MechanismsSynthesis and Biological Evaluation
Ni-Catalyzed Denitrogenative Cross-Coupling of Benzotriazinones and Cyclopropanols: An Easy Access to Functionalized β-Aryl Ketones | Litcius