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Electron Transport Assisted by Transparent Conductive Oxide Elements in Perovskite Solar Cells

Wenqi Zhang, Zhichao Lin, Qingbin Cai, Xiangning Xu, Hongye Dong, Cheng Mu, Jianping Zhang

2021ChemSusChem20 citationsDOI

Abstract

Abstract Fluorine and indium elements in F‐doped SnO 2 (FTO) and Sn‐doped In 2 O 3 (ITO), respectively, significantly contribute toward enhancing the electrical conductivity of these transparent conductive oxides. In this study, fluorine was combined with indium to modify the SnO 2 electron transport layer (ETL) through InF 3 . Consequently, the modified perovskite solar cells (PSCs) showe the favorable alignment of energy levels, improved absorption and utilization of light, enhanced interfacial charge extraction, and suppressed interfacial charge recombination. After InF 3 modification, the open circuit voltage ( V oc ) and fill factor (FF) of the PSC were significantly improved, and the photoelectric conversion efficiency (PCE) reached 21.39 %, far exceeding that of the control PSC (19.62 %).

Topics & Concepts

Materials sciencePerovskite (structure)DopingEnergy conversion efficiencyTransparent conducting filmOptoelectronicsPhotoelectric effectElectrical conductorIndiumOxideConductivityOpen-circuit voltageIndium tin oxideChemical engineeringLayer (electronics)NanotechnologyChemistryVoltageComposite materialPhysical chemistryMetallurgyQuantum mechanicsPhysicsEngineeringPerovskite Materials and ApplicationsConducting polymers and applicationsQuantum Dots Synthesis And Properties