Convergent paired electrosynthesis of dimethyl carbonate from carbon dioxide enabled by designing the superstructure of axial oxygen coordinated nickel single-atom catalysts
Xiaofang Li, Shu‐Guo Han, Weiming Wu, Kexin Zhang, Bo Chen, Shenghua Zhou, Dong-Dong Ma, Wenbo Wei, Xin‐Tao Wu, Ruqiang Zou, Qi‐Long Zhu
Abstract
A dual-channel superstructured Ni single-atom catalyst with a unique axial oxygen coordination configuration was controllably constructed and affords a preeminent performance for convergent paired electrosynthesis of dimethyl carbonate from CO 2 .
Topics & Concepts
ElectrosynthesisNickelCarbonateCatalysisSuperstructureDimethyl carbonateCarbon dioxideOxygen evolutionOxygen atomOxygenMaterials scienceAtom (system on chip)ChemistryChemical engineeringNanotechnologyElectrochemistryPhysical chemistryElectrodeMetallurgyOrganic chemistryPhysicsMoleculeThermodynamicsComputer scienceEmbedded systemEngineeringCO2 Reduction Techniques and CatalystsCarbon dioxide utilization in catalysisAdvanced battery technologies research