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New Design of Active Material Based on YInWO<sub>4</sub>-G-SiO<sub>2</sub>for a Urea Sensor and High Performance for Nonenzymatic Electrical Sensitivity

Kamrun Nahar Fatema, Chong‐Hun Jung, Yin Liu, Suresh Sagadevan, Kwang Youn Cho, Won‐Chun Oh

2020ACS Biomaterials Science & Engineering24 citationsDOI

Abstract

In the present study, electrochemical sensing for urea was proposed utilizing graphene-based quaternary nanocomposites YInWO4-G-SiO2 (YIWGS). These YIWGS nanocomposites were utilized due to their exceptionally delicate determination of urea with the lowest detection limit (0.01 mM). These YIWGS composites were developed through a simple self-assembly method. From physical characterization, we found that the YIWGS composites are crystalline in nature (powdered X-ray diffraction), and Fourier transform infrared (FTIR) spectroscopy analysis provided the surface functionality and bonding. Scanning electron microscopy (SEM) studies indicated the morphology characteristics of the as-synthesized composites and the high-resolution transmission electron microscopy (HRTEM) image supported the formation of cubic or hexagonal morphology of the YIW nanocomposites. The YIWGS sensor showed a great electroanalytical sensing performance of 0.07 mM urea with a sensitivity of 0.06 mA cm–2, an expansive linear range of 0.7–1.5 mM with a linear response (R2 1/4 0.99), and an eminent reaction time of around 2 s. It also displayed a good linear response toward urea with negligible interferences from normal coinciding species in urine samples.

Topics & Concepts

High-resolution transmission electron microscopyMaterials scienceNanocompositeFourier transform infrared spectroscopyScanning electron microscopeUreaDetection limitTransmission electron microscopyGrapheneLinear rangeAnalytical Chemistry (journal)Chemical engineeringNanotechnologyComposite materialChemistryOrganic chemistryChromatographyEngineeringElectrochemical sensors and biosensorsGas Sensing Nanomaterials and SensorsAnalytical Chemistry and Sensors