Litcius/Paper detail

Temperature Distribution in TaO<sub><i>x</i></sub> Resistive Switching Devices Assessed In Operando by Scanning Thermal Microscopy

Jingjia Meng, Jonathan M. Goodwill, Evgheni Strelcov, Kefei Bao, Jabez J. McClelland, Marek Skowroński

2023ACS Applied Electronic Materials10 citationsDOIOpen Access PDF

Abstract

High Resolution Image Download MS PowerPoint Slide Understanding the physical changes during electroformation and switching processes in transition-metal-oxide-based non-volatile memory devices is important for advancing this technology. Relatively few characteristics of these devices have been assessed in operando. In this work, we present scanning thermal microscopy measurements in vacuum on TaO x -based memory devices electroformed in both positive and negative polarities and high- and low-resistance states. The observed surface temperature footprints of the filament showed higher peak temperatures and narrower temperature distributions when the top electrode served as the anode in the electroformation process. This is consistent with a model in which a hot spot is created by a gap in the conducting filament that forms closest to the anode. A similar behavior was seen on comparing the high-resistance state to the low-resistance state, with the low-resistance footprint showing a lower peak and a larger width, consistent with the gap disappearing when the device is switched from high resistance to low resistance.

Topics & Concepts

Scanning thermal microscopyMaterials scienceMicroscopyScanning electron microscopeThermalScanning probe microscopyResistive touchscreenOptoelectronicsAnalytical Chemistry (journal)NanotechnologyAtomic force microscopyChemistryOpticsElectrical engineeringComposite materialPhysicsThermodynamicsEngineeringChromatographyAdvanced Memory and Neural ComputingFerroelectric and Negative Capacitance DevicesSemiconductor materials and devices