Formation and growth of sub-3 nm particles in megacities: impact of background aerosols
Chenjuan Deng, Runlong Cai, Chao Yan, Jun Zheng, Jingkun Jiang
Abstract
, not significantly different from that in clean environments. The relatively low growth rate and the high level of scavenging by background aerosols result in low survival of newly formed particles. The analyses also reinforce prior results on the need to correct conventional methods to adequately quantify the formation and growth rates when analyzing data from megacities with strong coagulation scavenging due to background aerosols. The conventional balance formula underestimates the formation rate of 1.5 nm particles, while the conventional appearance time method overestimates the growth rate of sub-3 nm particles. These findings highlight the governing role of background aerosols in urban NPF.