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Explainable machine learning-enabled dual-objective design of γ' phase characteristic parameters in γ'-strengthened Co-based superalloys

Linlin Sun, Qingshuang Ma, Chen Pei, Huiwen Yao, Xili Liu, Jie Xiong, Chenxi Liu, Huijun Li, Qiuzhi Gao

2025npj Computational Materials6 citationsDOIOpen Access PDF

Abstract

The high-temperature performance of Co-based superalloys is primarily dictated by the coarsening kinetics and volume fraction of the γ′ phase. To simultaneously optimize these two interrelated microstructural parameters, we propose a dual-objective design framework that integrates explainable machine learning (XML), multi-fidelity data augmentation, and SHapley Additive exPlanations (SHAP)-based interpretability. For γ′ phase coarsening rate constant ( K r ), a small experimental dataset was expanded using medium-fidelity simulations and further balanced with low-fidelity synthetic samples. For γ′ volume fraction ( V γ′ ), synthetic oversampling was applied to a larger dataset to mitigate distribution imbalance. ML models trained on these augmented datasets achieved high predictive accuracy, with SHAP analysis providing interpretable insights. Guided by these insights, several new compositions were proposed and validated. The optimal composition, Co-30Ni-10Al-3Ti-4Ta-5Cr-2Mo-1V (at.%), achieves a low K r of 0.756 ± 0.06 nm 2 ·s -1 and a high V γ′ of exceeding 70% at 1000 °C, while also fulfills multiple other critical design criteria, offering a promising route for next-generation Co-based superalloys.

Topics & Concepts

SuperalloyVolume fractionOversamplingFraction (chemistry)Constant (computer programming)Phase (matter)Volume (thermodynamics)Computer scienceDistribution (mathematics)Materials scienceArtificial intelligenceDesign of experimentsAlgorithmExperimental dataMathematicsHigh dimensionalHigh Temperature Alloys and CreepMicrostructure and Mechanical Properties of SteelsIntermetallics and Advanced Alloy Properties
Explainable machine learning-enabled dual-objective design of γ' phase characteristic parameters in γ'-strengthened Co-based superalloys | Litcius