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Single-photon emitters in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mi mathvariant="normal">WSe</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math>: Critical role of phonons on excitation schemes and indistinguishability

Luca Vannucci, José Ferreira Neto, Claudia Piccinini, Athanasios Paralikis, Niels Gregersen, Battulga Munkhbat

2024Physical review. B./Physical review. B11 citationsDOIOpen Access PDF

Abstract

Quantum emitters in few-layer WSe${}_{2}$ hold promise for scalable quantum computation. However, a significant challenge is to prepare the emitter in a specific excited state ``on-demand''. Here, the authors demonstrate that the emitter-phonon coupling has a crucial influence on the state preparation fidelity, because such a coupling is orders of magnitude stronger in WSe${}_{2}$ compared to other platforms. While excitation with resonant laser pulses is found to be significantly damped by phonons, alternative strategies based on detuned pulses allow for fast and reliable state preparation.

Topics & Concepts

ExcitationPhononPhotonPhysicsCondensed matter physicsTwo-photon excitation microscopyAtomic physicsQuantum mechanicsOrganic and Molecular Conductors Research2D Materials and ApplicationsMolecular Junctions and Nanostructures
Single-photon emitters in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mi mathvariant="normal">WSe</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math>: Critical role of phonons on excitation schemes and indistinguishability | Litcius