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Reductive Amination Routes in the Synthesis of Piperidine IminoSugars

Francesca Clemente, Camilla Matassini, Francesca Cardona

2020European Journal of Organic Chemistry25 citationsDOI

Abstract

The reductive amination (RA) reaction plays a pivotal role in the synthesis of new C–N bonds, due to the availability of many different and low‐cost reagents and their operational simplicity. The introduction in a compound of a nitrogen‐containing moiety that can be reduced to an amine in the reaction medium allows to perform cascade reactions which further expand this method. The application of the intramolecular version of the RA to carbohydrates allows the synthesis of polyhydroxypiperidine iminosugars, which are among the most challenging and fascinating glycomimetics for a synthetic chemist. This minireview focuses on the use of RA and of the double reductive amination (DRA) reaction in the key ring‐closing step en route to the synthesis of these compounds.

Topics & Concepts

Reductive aminationChemistryCombinatorial chemistryIntramolecular forceAminationIminosugarMoietyAmine gas treatingReagentPiperidineReductive eliminationCascade reactionOrganic chemistryCatalysisEnzymeCarbohydrate Chemistry and SynthesisChemical Synthesis and AnalysisSynthetic Organic Chemistry Methods
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