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Plasmon‐Driven Highly Selective CO<sub>2</sub> Photoreduction to C<sub>2</sub>H<sub>4</sub> on Ionic Liquid‐Mediated Copper Nanowires

Hongli Liu, Bin Sun, Zaiqi Li, Difei Xiao, Zeyan Wang, Yuanyuan Liu, Zhaoke Zheng, Peng Wang, Ying Dai, Hefeng Cheng, Baibiao Huang

2024Angewandte Chemie International Edition17 citationsDOIOpen Access PDF

Abstract

Abstract Selective CO 2 photoreduction to value‐added multi‐carbon (C 2+ ) feedstocks, such as C 2 H 4 , holds great promise in direct solar‐to‐chemical conversion for a carbon‐neutral future. Nevertheless, the performance is largely inhibited by the high energy barrier of C−C coupling process, thereby leading to C 2+ products with low selectivity. Here we report that through facile surface immobilization of a 1‐ethyl‐3‐methylimidazolium tetrafluoroborate (EMIM‐BF 4 ) ionic liquid, plasmonic Cu nanowires could enable highly selective CO 2 photoreduction to C 2 H 4 product. At an optimal condition, the resultant plasmonic photocatalyst exhibits C 2 H 4 production with selectivity up to 96.7 % under 450 nm monochromatic light irradiation, greatly surpassing its pristine Cu counterpart. Combined in situ spectroscopies and computational calculations unravel that the addition of EMIM‐BF 4 ionic liquid modulates the local electronic structure of Cu, resulting in its enhanced adsorption strength of *CO intermediate and significantly reduced energy barrier of C−C coupling process. This work paves new path for Cu surface plasmons in selective artificial photosynthesis to targeted products.

Topics & Concepts

NanowireCopperPlasmonIonic bondingIonic liquidMaterials scienceSurface plasmon resonanceNanotechnologyPhotochemistryIonOptoelectronicsNanoparticleChemistryCatalysisMetallurgyOrganic chemistryCO2 Reduction Techniques and CatalystsAdvanced Photocatalysis TechniquesCatalytic Processes in Materials Science