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Half-Metallic Heusler Alloy/MoS<sub>2</sub> Based Magnetic Tunnel Junction

Konstantin V. Larionov, Jose J. Pais Pereda, Songtian Li, Seiji Sakai, Павел Б. Сорокин

2022ACS Applied Materials & Interfaces10 citationsDOI

Abstract

Integration of half-metallic materials and 2D spacers into vertical magnetoresistive spin valves may pave the way for effective low-power consumption storage and memory technologies. Driven by the recent successful growth of graphene/half-metallic Co2Fe(Ge1/2Ga1/2) (CFGG) heterostructure, here we report a theoretical investigation of magnetic tunnel junction (MTJ) based on the ferromagnetic CFGG Heusler alloy and the MoS2 spacer of different thicknesses. Using ab initio approach, we demonstrate that the inherent ferromagnetism of CFGG is preserved at the interface, while its half-metallicity is recovering within few atomic layers. Ballistic transport in CFGG/MoS2/CFGG MTJ is studied within the nonequilibrium Green’s function formalism, and a large magnetoresistance value up to ∼105% is observed. These findings support the idea of effective spintronics devices based on half-metallic Heusler alloys and highly diversified transition metal dichalcogenide family.

Topics & Concepts

Materials scienceSpintronicsTunnel magnetoresistanceCondensed matter physicsFerromagnetismMagnetoresistanceHeterojunctionGrapheneAlloyNanotechnologyOptoelectronicsMagnetic fieldMetallurgyPhysicsQuantum mechanics2D Materials and ApplicationsFerroelectric and Negative Capacitance DevicesMagnetic properties of thin films
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