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Accelerated Newton-Raphson GRAPE methods for optimal control

David L. Goodwin, Mads Sloth Vinding

2023Physical Review Research20 citationsDOIOpen Access PDF

Abstract

Improvements to the optimal control Newton-Raphson GRAPE method for exact Hessian calculations are shown with examples of auxiliary matrix and ESCALADE methods. For an ensemble of two-level systems with realistic MRI conditions, the new accelerated Hessian calculations are between 200 and 600 times faster for auxiliary matrix and ESCALADE, respectively.

Topics & Concepts

Hessian matrixNewton's methodOptimal controlMatrix (chemical analysis)Quasi-Newton methodMathematicsApplied mathematicsHessian equationMathematical optimizationComputer sciencePhysicsMathematical analysisChemistryNonlinear systemChromatographyQuantum mechanicsFirst-order partial differential equationPartial differential equationAdvanced NMR Techniques and ApplicationsAdvanced MRI Techniques and ApplicationsNMR spectroscopy and applications