Litcius/Paper detail

Role of KCl in activation mechanisms of KOH-chemically activated high surface area carbons

Ignacio Campello Gómez, Orlando F. Cruz, Joaquín Silvestre‐Albero, Carlos R. Rambo, Manuel Martínez Escandell

2022Journal of CO2 Utilization40 citationsDOIOpen Access PDF

Abstract

Activated carbons from different precursors have been synthetized using KOH and mixtures of KOH and KCl as activating agents. The results revealed an increase of surface area and yield of activation related with KCl addition in all the samples. Thermodynamic and mass spectrometry studies reveal that KCl do not act as an activating agent, but promotes the solubilisation of secondary products of the reactions such as carbonates, enhancing the contact of KOH and carbon particles, therefore increasing the efficiency of the activation. Based on mass spectroscopy results, combined with thermodynamic calculations, we proposed four reactions as the most likely responsible for the pore development during activation.

Topics & Concepts

Yield (engineering)ChemistryActivated carbonMass spectrometryChemical engineeringCarbon fibersMaterials scienceOrganic chemistryChromatographyAdsorptionMetallurgyEngineeringComposite materialComposite numberZeolite Catalysis and SynthesisCovalent Organic Framework ApplicationsCatalytic Processes in Materials Science