Bending two-dimensional Cu(<scp>i</scp>)-based coordination networks to inverse electrocatalytic HER/CO<sub>2</sub>RR selectivity
Kai Zheng, Ding-Yi Hu, Xuewen Zhang, Xian-Xian Xiao, Zi-Jun Liang, Jun Wu, Duoyu Lin, Lin‐Ling Zhuo, Yi Heng, Gong Li, Dong‐Dong Zhou, Jie‐Peng Zhang
Abstract
By introducing an amino group on the ligand, the shape of two-dimensional coordination polymers transforms from planar into wavy, creating a supramolecular microenvironment to boost the CO 2 RR for C 2 H 4 and simultaneously restrict the HER.
Topics & Concepts
SelectivityBendingInverseChemistryMaterials scienceComputer sciencePhysicsComposite materialCatalysisMathematicsGeometryBiochemistryCO2 Reduction Techniques and CatalystsCovalent Organic Framework ApplicationsIonic liquids properties and applications