Atmosphere-directed reconstruction of Cu-based metal–organic frameworks toward efficient CO<sub>2</sub> electroreduction
Jiye Feng, Danni Shi, Fei Wang, Yiming Zou, Weicheng Li, Wenbiao Zhang, Huaijun Lin, Yuying Meng, Qingsheng Gao
Abstract
coordination, remains stable, highlighting the framework-dependent nature. These findings establish atmosphere-controlled reconstruction of metastable MOFs as a powerful tool for rational electrocatalyst design.
Topics & Concepts
ElectrochemistryRedoxValence (chemistry)MetalChemisorptionChemistryReducing atmosphereAdsorptionAtmosphere (unit)Metal-organic frameworkChemical engineeringMaterials scienceInorganic chemistryNanotechnologyElectrodePhysical chemistryOrganic chemistryThermodynamicsPhysicsEngineeringCO2 Reduction Techniques and CatalystsIonic liquids properties and applicationsMetal-Organic Frameworks: Synthesis and Applications