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Pb2+ removal performance by cotton-based and magnetic modified cotton-based biochar prepared from agricultural waste biomass

Yan-ling Zou, F. Z. Xu, Qiang Kong, Dawei Shang, Yujia Zhang, Wenhan Guo, Qian Wang, Congcong Zhao, Yuanda Du

2020Desalination and Water Treatment11 citationsDOIOpen Access PDF

Abstract

ABSTRACT This study aimed to investigate the Pb 2+ removal performance of cotton-based biochar (CB) and magnetic modified cotton-based biochar (MCB). The scanning electron microscopy revealed that MCB exhibiting a porous honeycomb structure with a specific surface area of 613.69 m 2 /g which bigger than that of CB (356.68 m 2 /g). The Fourier transform infrared spectrum analysis indicated the presence of metal oxides and hydroxides in MCB and the functional groups of O–H, C=O, and C≡C in both MCB and CB. The signal of Fe 3 O 4 and Fe 3 C was observed in X-ray diffraction analysis of MCB, which indicated the success of magnetic modification of MCB. The maximum monolayer adsorption capacities (Q m ) of MCB and CB on Pb 2+ were 208.33 and 156.25 mg/g, respectively. The adsorption kinetics of MCB and CB were both best fitted with the pseudo-second-order model (R 2 > 0.99), and the adsorption isotherms of the two biochar were well-described by the Langmuir adsorption model (R 2 > 0.99). The results of this study revealed the significant physicochemical difference of two biochar and indicated that magnetic modification can enhance the Pb 2+ adsorption capacity of biochar, suggesting that MCB is a potential adsorbent for wastewater treatment.

Topics & Concepts

BiocharAdsorptionFourier transform infrared spectroscopyLangmuir adsorption modelChemistryNuclear chemistryMonolayerBiomass (ecology)Specific surface areaScanning electron microscopeWastewaterChemical engineeringMaterials scienceWaste managementCatalysisOrganic chemistryComposite materialAgronomyPyrolysisBiochemistryEngineeringBiologyAdsorption and biosorption for pollutant removalFluoride Effects and RemovalPhosphorus and nutrient management