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Strongly correlated superconductivity in a copper-based metal-organic framework with a perfect kagome lattice

Takaaki Takenaka, K. Ishihara, M. Roppongi, Yijie Miao, Yuta Mizukami, T. Makita, Junto Tsurumi, Shun Watanabe, J. Takeya, Minoru Yamashita, Kenji Torizuka, Yoshiya Uwatoko, T. Sasaki, Xing Huang, W. Xu, Daoben Zhu, Ninghu Su, Jinguang Cheng, T. Shibauchi, K. Hashimoto

2021Science Advances100 citationsDOIOpen Access PDF

Abstract

of 0.25 kelvin raises fundamental questions about the nature of electron pairing. Here, we show that Cu-BHT is a strongly correlated unconventional superconductor with extremely low superfluid density. A nonexponential temperature dependence of superfluid density is observed, indicating the possible presence of superconducting gap nodes. The magnitude of superfluid density is much smaller than those in conventional superconductors and follows the Uemura's relation of strongly correlated superconductors. These results imply that the unconventional superconductivity in Cu-BHT originates from electron correlations related to spin fluctuations of kagome lattice.

Topics & Concepts

SuperconductivitySuperfluidityCondensed matter physicsPhysicsFrustrationPairingLattice (music)Electron pairMetalCopperOrganic superconductorSpin (aerodynamics)QuantumElectronMaterials scienceQuantum mechanicsThermodynamicsAcousticsMetallurgyAdvanced Condensed Matter PhysicsPhysics of Superconductivity and MagnetismOrganic and Molecular Conductors Research