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Electrocatalytic selectivity for nitrogen reduction <i>vs.</i> hydrogen evolution: a comparison of vanadium and cobalt oxynitrides at different pH values

Precious Chukwunenye, Ashwin Ganesan, Mojgan Gharaee, Kabirat Balogun, Fatima Anwar, Qasim Adesope, Thomas R. Cundari, Francis D’Souza, Jeffry A. Kelber

2022Journal of Materials Chemistry A23 citationsDOI

Abstract

To understand the competing HER and NRR reactions, their selectivities are compared for well-known NRR catalysts, viz. , metal oxynitrides of high (vanadium) and low (cobalt) oxophilicity as a function of pH.

Topics & Concepts

CobaltVanadiumInorganic chemistrySelectivityCatalysisMetalNitrogenHydrogenChemistryRedoxMaterials scienceOrganic chemistryAmmonia Synthesis and Nitrogen ReductionElectrocatalysts for Energy ConversionAdvanced Photocatalysis Techniques