Directly revealing the geometric phase effect of dissociative D<sub>2</sub><sup>+</sup>by two-color strong field photodissociation
Zhaopeng Sun, Liu Yunquan
Abstract
with the random orientation by solving the time-dependent Schrödinger equation. We reveal the GP effect that manifests as the Aharonov-Bohm-like interference in the photofragment angular distribution along the direction perpendicular to the linear polarization axis. Our work deepens the understanding of the physical mechanisms of the molecular dynamics when driven by the synthesized strong laser field.
Topics & Concepts
Conical intersectionPhotodissociationGeometric phaseLinear polarizationPolarization (electrochemistry)Angular momentumAtomic physicsPhysicsPerpendicularLaserHigh harmonic generationWave functionField (mathematics)ElectronChemistryQuantum mechanicsExcited stateGeometryPhotochemistryMathematicsPure mathematicsPhysical chemistryLaser-Matter Interactions and ApplicationsSpectroscopy and Quantum Chemical StudiesAdvanced Chemical Physics Studies