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Chiral Resolution of Mandelic Acid through Preferential Cocrystallization with Nefiracetam

Xavier Buol, Camila Caro Garrido, Koen Robeyns, Nikolay Tumanov, Laurent Collard, Johan Wouters, Tom Leyssens

2020Crystal Growth & Design47 citationsDOIOpen Access PDF

Abstract

In this paper, we identified a cocrystal conglomerate of mandelic acid using a drug compound as a coformer. We then developed a chiral resolution process based on preferential cocrystallization. Several versions of such a process were explored and optimized, leading to a successful resolution of mandelic acid, evidencing the efficiency of our system. Excellent enantiopurity (98–99%) was obtained with a process that can run for multiple cycles.

Topics & Concepts

Mandelic acidCocrystalChemistryResolution (logic)Chiral resolutionProcess (computing)Combinatorial chemistryStereochemistryOrganic chemistryEnantiomerHydrogen bondMoleculeComputer scienceOperating systemArtificial intelligenceCrystallization and Solubility StudiesCrystallography and molecular interactionsAnalytical Chemistry and Chromatography