Litcius/Paper detail

Novel High-Temperature Alkaline Water Electrolysis Using Molten KOH–H<sub>2</sub>O System

Kenji Kawaguchi, Keita Goto, Aozora Konno, Toshiyuki Nohira

2023Journal of The Electrochemical Society10 citationsDOIOpen Access PDF

Abstract

To improve water electrolysis efficiency, we investigated the hydrogen and oxygen evolution reactions (HER and OER) at a Ni electrode in a molten KOH–H 2 O system (85:15 wt%, 65:35 mol%) at a high temperature (150 °C). The overpotentials for the HER and OER at 500 mA cm −2 were significantly reduced, by 261 mV and 75 mV, respectively, in the novel system relative to those obtained in a conventional aqueous solution system (30 wt% KOH, 80 °C). The decreases in polarization were attributed predominantly to kinetic effects, including a change in the rate-determining steps, on the HER and OER with the change of electrolytes.

Topics & Concepts

Oxygen evolutionElectrolysisAlkaline water electrolysisElectrolyteElectrolysis of waterChemistryAqueous solutionElectrochemistryPolarization (electrochemistry)Inorganic chemistryMolten saltElectrodeAnalytical Chemistry (journal)Physical chemistryChromatographyAdvancements in Solid Oxide Fuel CellsElectrocatalysts for Energy ConversionAdvanced battery technologies research