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Temperature-induced dephasing in high-order harmonic generation from solids

Tao-Yuan Du, Chao Ma

2022Physical review. A/Physical review, A31 citationsDOIOpen Access PDF

Abstract

High-order harmonic generation (HHG) in solid and gaseous targets has been proven to be a powerful avenue for the generation of attosecond pulses, whereas the influence of electron-phonon scattering on HHG is a critical outstanding problem. Here we first introduce a temperature-dependent lattice vibration model by characterizing the spacing fluctuation. Our results reveal that (i) structural disorder induced by lattice vibration does not lead to generation of even-order harmonics; (ii) dephasing of HHG occurs as the lattice temperature is growing; (iii) an open-trajectory picture predicts the maximal photon energy in the temperature-dependent HHG spectra. Moreover, a formula assessing dephasing time with lattice temperature is proposed to identify the timescale of electron-phonon scattering. This work paves the way to study the non-Born-Oppenheimer effect in solids driven by a strong field.

Topics & Concepts

DephasingHarmonicsHigh harmonic generationPhysicsPhononScatteringCondensed matter physicsElectronAttosecondLattice (music)PhotonAtomic physicsQuantum mechanicsLaserUltrashort pulseAcousticsVoltageLaser-Matter Interactions and ApplicationsTerahertz technology and applicationsLaser-Plasma Interactions and Diagnostics
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