Litcius/Paper detail

Distal Ruthenaelectro‐Catalyzed <i>meta</i> ‐C−H Bromination with Aqueous HBr

Yulei Wang, Hendrik Simon, Xinran Chen, Zhipeng Lin, Shan Chen, Lutz Ackermann

2022Angewandte Chemie International Edition47 citationsDOIOpen Access PDF

Abstract

Abstract While electrochemical ortho ‐selective C−H activations are well established, distal C−H activations continue to be underdeveloped. In contrast, we herein describe the electrochemical meta ‐C−H functionalization. The remote C−H bromination was accomplished in an undivided cell by RuCl 3 ⋅3 H 2 O with aqueous HBr. The electrohalogenation proceeded under exogenous ligand‐ and electrolyte‐free conditions. Notably, pyrazolylarenes were meta ‐selectively brominated at the benzenoid moiety, rather than on the electron‐rich pyrazole ring for the first time. Mechanistic studies were suggestive of an initial ruthenacycle formation, and a subsequent ligand‐to‐ligand hydrogen transfer (LLHT) process to liberate the brominated product.

Topics & Concepts

HalogenationCatalysisAqueous solutionChemistryMedicinal chemistryOrganic chemistryCatalytic C–H Functionalization MethodsAsymmetric Hydrogenation and CatalysisCatalytic Cross-Coupling Reactions