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One-Pot Synthesis of Symmetrical and Asymmetrical 3-Amino Diynes via Cu(I)-Catalyzed Reaction of Enaminones with Terminal Alkynes

Changyuan Zhang, Huosheng Guo, Lulu Chen, Jiantao Zhang, Mengping Guo, Xuncheng Zhu, Chan Moh. Shen, Li Zeng

2021Organic Letters15 citationsDOI

Abstract

An economical and efficient protocol for the direct construction of amino skipped diynes through the Cu(I)-catalyzed reaction of enaminones and terminal alkynes has been described. Different kinds of symmetrical and asymmetrical 3-amino diynes could be obtained in up to 83% yield through a one-pot reaction under mild conditions.

Topics & Concepts

ChemistryYield (engineering)CatalysisTerminal (telecommunication)Reaction conditionsAmino acidCombinatorial chemistryStereochemistryOrganic chemistryBiochemistryPhysicsTelecommunicationsComputer scienceThermodynamicsCatalytic Alkyne ReactionsCatalytic C–H Functionalization MethodsSynthesis and Characterization of Pyrroles