Advances and challenges of metal organic frameworks (MOFs) and derivatives in photoelectrocatalytic water splitting
Xin-Jie Tian, Sijia Guo, Zhengyi Wu, Na Xu, Guan‐Qun Han, Yong‐Ming Chai, Bin Dong
Abstract
ligand bonds. They offer high specific surface areas, abundant metal active sites, large pore volumes, and customizable structures and compositions, making them highly favorable for applications in photoelectrocatalysis. This review discusses the advancements in photoelectrocatalytic hydrogen production technology using metal-organic frameworks (MOFs) and derivatives. It covers the principles of photoelectrocatalysis, preparation methods for MOF catalysts and strategies for performance enhancement. These strategies include improving light absorption, enhancing carrier separation efficiency, and ensuring stability. The paper also discusses the current challenges and future directions of photoelectrocatalytic water splitting technology. Overall, this review offers a thorough theoretical framework and practical insights for researchers in this field.