Litcius/Paper detail

Boryl radical-mediated halogen-atom transfer (XAT) enables the Sonogashira-like alkynylation of alkyl halides

Javier Corpas, Maialen Alonso, Daniele Leonori

2024Chemical Science28 citationsDOIOpen Access PDF

Abstract

The Sonogashira-like alkynylation of alkyl halides is achieved by a photocatalytic approach exploiting amine-ligated boryl radicals as halogen-atom transfer mediators in combination with alkynyl sulfones as SOMOphilic reagents.

Topics & Concepts

Sonogashira couplingAlkynylationHalideAlkylHalogenChemistryAtom (system on chip)Combinatorial chemistryOrganic chemistryCatalysisPalladiumComputer scienceEmbedded systemRadical Photochemical ReactionsCatalytic C–H Functionalization MethodsCatalytic Cross-Coupling Reactions