Litcius/Paper detail

Asymmetric Catalytic Ring‐Expansion of 3‐Methyleneazetidines with α‐Diazo Pyrazoamides towards Proline‐Derivatives

Kaixuan Wang, Longqing Yang, Yi Li, Hongye Li, Zhili Liu, Lichao Ning, Xiaohua Liu, Xiaoming Feng

2023Angewandte Chemie International Edition22 citationsDOIOpen Access PDF

Abstract

We realized a highly efficient formal [1,2]-sigmatropic rearrangement of ammonium ylides generated from 3-methylene-azetidines and α-diazo pyrazoamides. The employ of readily available chiral cobalt(II) complex of chiral N,N'-dioxide enabled the ring-expansion of azetidines, affording a variety of quaternary prolineamide derivatives with excellent yield (up to 99 %) and enantioselectivity (up to 99 % ee) under mild reaction condition. For the rearrangement of ammonium ylides, the installation of a pyrazoamide group as a masked brick to build chiral scaffolds proved successful. The enantioselective ring expansion process was elucidated by DFT calculations.

Topics & Concepts

DiazoEnantioselective synthesisRing (chemistry)ChemistryYield (engineering)MethyleneSigmatropic reactionAziridineCatalysisAmmoniumMedicinal chemistryCombinatorial chemistryOrganic chemistryMaterials scienceMetallurgySynthesis and Catalytic ReactionsCyclopropane Reaction MechanismsSynthesis of β-Lactam Compounds