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Femtosecond laser regulatory focus ablation patterning of a fluorescent film up to 1/10 of the scale of the diffraction limit

Shuyu Liang, Yue‐Feng Liu, Jian‐Guan Hua, Zhi‐Kun Ji, Hong Xia

2023Nanoscale13 citationsDOI

Abstract

Patterned quantum dots (QDs) and perovskites have attracted a great deal of attention in the fabrication of optoelectronic device arrays for transistors, image sensors and displays. However, the resolution of current patterning technologies is insufficient for nanopatterned QDs and perovskites to be integrated in advanced optoelectronic and photonic applications. Herein, we demonstrate a femtosecond laser regulatory focus ablation (FsLRFA) patterning technique of a fluorescent film involving both semiconductor core-shell QDs and perovskite up to 1/10th of the scale of the diffraction limit. Annular lines with a 200 nm-width are obtained after the irradiation of the femtosecond laser. Moreover, the combination of ablated different geometries enables the laser focal spot as brushes for FsLRFA patterning technology to fabricate delicate and programmable patterns on the fluorescent film. This technology with nanoscale resolution and patterning capability paves the road toward highly integrated applications based on QDs and perovskites.

Topics & Concepts

FemtosecondMaterials scienceLaserNanotechnologyOptoelectronicsQuantum dotFabricationDiffractionNanoscopic scaleLaser ablationPhotonicsPerovskite (structure)OpticsChemistryAlternative medicineMedicinePathologyCrystallographyPhysicsNonlinear Optical Materials StudiesLaser Material Processing TechniquesNear-Field Optical Microscopy
Femtosecond laser regulatory focus ablation patterning of a fluorescent film up to 1/10 of the scale of the diffraction limit | Litcius