Litcius/Paper detail

Catalytic Activation of Polyethylene Model Compounds Over Metal‐Exchanged Beta Zeolites

Jacob H. Miller, Anne K. Starace, Daniel A. Ruddy

2022ChemSusChem24 citationsDOIOpen Access PDF

Abstract

Abstract Decomposition of polymers by heterogeneous catalysts presents a promising approach for reuse of waste plastics. We demonstrated non‐hydrogenative decomposition of model polyolefins over proton‐form and metal (Cu, Ni) ion‐exchanged beta (BEA) zeolites at moderate temperatures (around 300 °C). Near complete polyolefin decomposition was observed in batch reactions monitored by thermogravimetric analysis, while decomposition at partial conversion was studied in flow reactions. Ni‐exchanged zeolites produced H 2 at substantially higher rates (>10x) than other catalysts while also uniquely resisting deactivation over time. Application of the delplot formalism offered insights into the reaction network for polyolefin decomposition over Ni/BEA most notably that H 2 is solely a primary product. We deduce that H 2 production is catalyzed by activation of C−H bonds at ionic Ni sites, and H 2 prevents buildup of polyaromatic coke species in Ni‐exchanged zeolites that deactivate Cu‐exchanged and protonic zeolites.

Topics & Concepts

CatalysisPolyolefinDecompositionChemistryZeoliteThermogravimetric analysisInorganic chemistryCokeMetalOrganic chemistryLayer (electronics)Zeolite Catalysis and SynthesisCarbon dioxide utilization in catalysisPolymer crystallization and properties