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Ubiquitous spin freezing in the superconducting state of UTe2

Shyam Sundar, N. Azari, M. R. Goeks, Shayan Gheidi, M. Abedi, Michael Yakovlev, S. R. Dunsiger, J. M. Wilkinson, Stephen J. Blundell, Tristin Metz, Ian Hayes, Shanta Saha, Sangyun Lee, Andrew Woods, R. Movshovich, S. M. Thomas, Nicholas P. Butch, P. F. S. Rosa, Johnpierre Paglione, J. E. Sonier

2023Communications Physics26 citationsDOIOpen Access PDF

Abstract

Abstract In most superconductors electrons form Cooper pairs in a spin-singlet state mediated by either phonons or by long-range interactions such as spin fluctuations. The superconductor UTe 2 is a rare material wherein electrons are believed to form pairs in a unique spin-triplet state with potential topological properties. While spin-triplet pairing may be mediated by ferromagnetic or antiferromagnetic fluctuations, experimentally, the magnetic properties of UTe 2 are unclear. By way of muon spin rotation/relaxation (μSR) measurements on independently grown UTe 2 single crystals we demonstrate the existence of magnetic clusters that gradually freeze into a disordered spin frozen state at low temperatures. Our findings suggest that inhomogeneous freezing of magnetic clusters is linked to the ubiquitous residual linear term in the temperature dependence of the specific heat ( C ) and the low-temperature upturn in C / T versus T . The omnipresent magnetic inhomogeneity has potential implications for experiments aimed at establishing the intrinsic low-temperature properties of UTe 2 .

Topics & Concepts

Muon spin spectroscopyCondensed matter physicsAntiferromagnetismSuperconductivityPairingSpin (aerodynamics)FerromagnetismSinglet stateElectronPhysicsCooper pairRelaxation (psychology)Triplet stateQuantum mechanicsExcited stateSocial psychologyThermodynamicsPsychologyRare-earth and actinide compoundsAdvanced Condensed Matter PhysicsMagnetic and transport properties of perovskites and related materials
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