Litcius/Paper detail

Metal-catalysed non-directed C(sp<sup>2</sup>)–H bond activation

Shubham Agrawal, Sandip Porey, Yogesh Bairagi, S.K. Maiti, Alex C. Bissember, Debabrata Maiti

2025Chemical Society Reviews19 citationsDOI

Abstract

)-H functionalization, with particular focus on both metal-catalyzed and metal-free systems. We examine notable progress in reaction scope, selectivity, and mechanistic insights, all of which highlight the strategic potential of these methods in the synthesis of complex molecules. Moreover, we discuss ongoing challenges, such as issues related to regioselectivity and substrate scope, while presenting potential avenues for improving the efficiency, sustainability, and applicability of non-directed C-H activation. The goal of this review is to provide a comprehensive picture of the current state of the field, aid understanding, and inspire further innovation in non-directed C-H functionalization as a versatile tool for advanced molecular design.

Topics & Concepts

Surface modificationCatalysisChemistryTransition metalMetalLigand (biochemistry)Combinatorial chemistryStereochemistryOrganic chemistryPhysical chemistryReceptorBiochemistryCatalytic C–H Functionalization MethodsSynthesis and Catalytic ReactionsCatalytic Cross-Coupling Reactions