Litcius/Paper detail

A chemical dynamics study on the gas-phase formation of triplet and singlet C <sub>5</sub> H <sub>2</sub> carbenes

Chao He, Galiya R. Galimova, Yuheng Luo, Long Zhao, André K. Eckhardt, Rui Sun, Alexander M. Mebel, Ralf I. Kaiser

2020Proceedings of the National Academy of Sciences25 citationsDOIOpen Access PDF

Abstract

) carbene-via the elementary reaction of the simplest organic radical-methylidyne (CH)-with diacetylene (HCCCCH) under single-collision conditions. Our combination of crossed molecular beam data with electronic structure calculations and quasi-classical trajectory simulations reveals fundamental reaction mechanisms and facilitates an intimate understanding of bond-breaking processes and isomerization processes of highly reactive hydrocarbon intermediates. The agreement between experimental chemical dynamics studies under single-collision conditions and the outcome of trajectory simulations discloses that molecular beam studies merged with dynamics simulations have advanced to such a level that polyatomic reactions with relevance to extreme astrochemical and combustion chemistry conditions can be elucidated at the molecular level and expanded to higher-order homolog carbenes such as butadiynylcyclopropenylidene and triplet heptatriynylidene, thus offering a versatile strategy to explore the exotic chemistry of novel higher-order carbenes in the gas phase.

Topics & Concepts

ChemistrySinglet stateReactive intermediateReaction dynamicsCarbeneCrossed molecular beamChemical physicsComputational chemistryReaction intermediateIsomerizationChemical reactionMolecular dynamicsPhotochemistryMoleculeAtomic physicsPhysicsOrganic chemistryExcited stateCatalysisAdvanced Chemical Physics StudiesChemical Reactions and MechanismsSynthesis and Properties of Aromatic Compounds