Photo-assisted high performance single atom electrocatalysis of the N<sub>2</sub> reduction reaction by a Mo-embedded covalent organic framework
Juan Wang, Zhihua Zhang, Siyun Qi, Yingcai Fan, Yanmei Yang, Weifeng Li, Mingwen Zhao
Abstract
Through theoretical calculations, we report the remarkably high catalytic activity and excellent selectivity of Mo-doped Pc-TFPN COF for the N 2 fixation and reduction reaction under ambient conditions.
Topics & Concepts
ElectrocatalystSelectivityCovalent bondCatalysisReduction (mathematics)Atom (system on chip)Materials scienceChemistryCovalent organic frameworkOxygen reduction reactionPhotochemistryPhysical chemistryElectrochemistryElectrodeOrganic chemistryComputer scienceMathematicsGeometryEmbedded systemAmmonia Synthesis and Nitrogen ReductionAdvanced Photocatalysis TechniquesCovalent Organic Framework Applications