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A Deep-Red Emission Phosphor Y<sub>2</sub>SrAl<sub>4</sub>SiO<sub>12</sub>:Ce<sup>3+</sup>, Cr<sup>3+</sup> and Its Utilization in Polycrystalline Silicon Solar Cells

Xiongbo Ma, Takatoshi Seto, Yuhua Wang

2023The Journal of Physical Chemistry Letters32 citationsDOI

Abstract

The power conversion efficiency (PCE) of crystalline silicon solar cells has reached a bottleneck. Further improving the PCE is an important current research topic. This Letter reports a new phosphor Y 2 SrAl 4 SiO 12:Ce 3+, Cr 3+ . Under the excitation in the wavelength range of 320–650 nm, the phosphor Y 2 SrAl 4 SiO 12:Ce 3+, Cr 3+ exhibits a deep-red emission in the 500–800 nm range. Due to the energy transfer from Ce 3+ to Cr 3+, the luminescence intensity of Cr 3+ is further enhanced. This matches well with the spectrum of silicon solar cells. Because of the powerful absorption and high internal quantum efficiency, Y 2 SrAl 4 SiO 12:Ce 3+, Cr 3+ was used to prepare energy down-conversion (EDC) films. By applying the EDC film on the surface of silicon solar cells, the relative PCE increases by 2.018%. These results indicate that Y 2 SrAl 4 SiO 12:Ce 3+, Cr 3+ is an excellent deep-red garnet structured phosphor and furthermore has a positive effect on the enhancement of the PCE of solar cells.

Topics & Concepts

PhosphorSiliconQuantum efficiencyMaterials scienceEnergy conversion efficiencyOptoelectronicsLuminescenceAbsorption (acoustics)Solar cellAnalytical Chemistry (journal)ChemistryChromatographyComposite materialLuminescence Properties of Advanced MaterialsGlass properties and applicationsPerovskite Materials and Applications
A Deep-Red Emission Phosphor Y<sub>2</sub>SrAl<sub>4</sub>SiO<sub>12</sub>:Ce<sup>3+</sup>, Cr<sup>3+</sup> and Its Utilization in Polycrystalline Silicon Solar Cells | Litcius