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Spectroscopic characterization for new complexes with 2,2′‐(5,5‐dimethylcyclohexane‐1,3‐diylidene)bis(azan‐1‐yl‐1‐ylidene)dibenzoic acid

Noor Mohamed Wannas, Abbas Ali Salih Al‐Hamdani, Wail Al Zoubi

2020Journal of Physical Organic Chemistry25 citationsDOI

Abstract

Abstract New series of metal ions complexes have been prepared from the new ligand [2,2′‐(5,5‐dimethylcyclohexane‐1,3‐diylidene)bis(azan‐1‐yl‐1‐ylidene)dibenzoic acid] derived from 5,5‐dimethylcyclohexane‐1,3‐dione and 2‐aminobenzoic acid. Accordingly, mono‐nuclear Ni(II), Pd(II), Re (II), and Pt(IV) complexes were prepared by the reaction of previous ligand with NiCl 2 .6H 2 O, PdCl 2 , ReCl 5 , and H 2 PtCl 6 .6H 2 O, respectively. The compounds have been characterized by Fourier‐transform infrared (FTIR), ultraviolet–visible (UV–vis), mass, H 1 ‐, and C 13 ‐nuclear magnetic resonance (NMR) spectra and thermo gravimetric analysis (TGA) curve, Bohr magnetic (B.M.), elemental microanalyses, metal ions, chloride containing, and molar conductance. These reviews uncovered octahedral geometries for the Re(V) and Pt (IV) complexes and tetrahedral for Ni (II) complex and square planer for Pd (II) complex. The investigation of complexes development by means at molar proportion and occupation strategy in DMF solution has been researched, and results were reliable to those found in the solid complexes with a proportion of (M:L) as (1:1).

Topics & Concepts

ChemistryOctahedronLigand (biochemistry)Proton NMRMetalChlorideNuclear chemistryMetal ions in aqueous solutionFourier transform infrared spectroscopyInfrared spectroscopyElemental analysisMedicinal chemistryInorganic chemistryCrystallographyStereochemistryCrystal structureOrganic chemistryBiochemistryQuantum mechanicsPhysicsReceptorMetal complexes synthesis and propertiesMagnetism in coordination complexesSynthesis and Reactivity of Heterocycles