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Calculation of absolute molecular entropies and heat capacities made simple

Philipp Pracht, Stefan Grimme

2021Chemical Science197 citationsDOIOpen Access PDF

Abstract

. Comprehensive tests indicate a relatively strong variation of the conformational entropy on the underlying level of theory for typical drug molecules, inferring the complex potential energy surfaces as the main source of error. Furthermore, we show some application examples for the calculation of free energy differences in typical chemical reactions.

Topics & Concepts

Simple (philosophy)Absolute (philosophy)Absolute zeroThermodynamicsMathematicsChemistryPhysicsPhilosophyEpistemologyChemical Thermodynamics and Molecular StructureAdvanced Thermodynamics and Statistical Mechanicsthermodynamics and calorimetric analyses