Litcius/Paper detail

Electron-phonon scattering in <b> <i>β</i> </b>-Ga2O3 studied by ultrafast transmission spectroscopy

S. Marcinkevičius, James S. Speck

2021Applied Physics Letters12 citationsDOIOpen Access PDF

Abstract

Femtosecond pump-probe experiments in a transmission geometry were performed on Sn-doped n-type β-Ga2O3. With the pump and probe wavelengths below the bandgap, the differential transmission signal was determined by the free electron dynamics. Differential transmission decay times and their spectral dependence were used to evaluate electron-phonon scattering for polar optical (PO) and intervalley phonons. The obtained average electron-PO phonon scattering time is 4.5 ± 0.4 fs, while the electron scattering to and from the side valley is 80 ± 5 fs. The energy between the absolute and second lowest conduction band minima is estimated to be 2.6 ± 0.1 eV.

Topics & Concepts

ScatteringPhononFemtosecondSpectroscopyAtomic physicsElectronPhonon scatteringPhotothermal spectroscopyMolecular physicsPhysicsChemistryMaterials scienceCondensed matter physicsOpticsLaserQuantum mechanicsGa2O3 and related materialsZnO doping and propertiesElectronic and Structural Properties of Oxides