Two-dimensional metal–organic framework Mo<sub>3</sub>(C<sub>2</sub>O)<sub>12</sub> as a promising single-atom catalyst for selective nitrogen-to-ammonia conversion
Zhen Feng, Zelin Yang, Xiaowen Meng, Fachuang Li, Zhanyong Guo, Zheng Shu, Guang Su, Yaqiang Ma, Yanan Tang, Xianqi Dai
Abstract
2D MOF Mo 3 (C 2 O) 12 not only possesses sufficient stability, but also exhibits high NRR activity with a low limiting potential of −0.36 V and substantial selectivity with a promising theoretical faradaic efficiency value of 100%.
Topics & Concepts
SelectivityFaraday efficiencyCatalysisLimitingNitrogenAmmoniaInorganic chemistryMetalMaterials scienceNitrogen atomAtom (system on chip)ChemistryAnalytical Chemistry (journal)Physical chemistryElectrodeElectrochemistryOrganic chemistryMetallurgyRing (chemistry)Embedded systemComputer scienceMechanical engineeringEngineeringAmmonia Synthesis and Nitrogen ReductionAdvanced Photocatalysis TechniquesMetal-Organic Frameworks: Synthesis and Applications