Litcius/Paper detail

Oxidation and Reduction of Polycrystalline Cerium Oxide Thin Films in Hydrogen

Adva Ben Yaacov, Lorenz J. Falling, Roey Ben David, Smadar Attia, Miguel Andrés, Slavomír Nemšák, Baran Eren

2023The Journal of Physical Chemistry Letters11 citationsDOIOpen Access PDF

Abstract

High Resolution Image Download MS PowerPoint Slide This study investigates the oxidation state of ceria thin films’ surface and subsurface under 100 mTorr hydrogen using ambient pressure X-ray photoelectron spectroscopy. We examine the influence of the initial oxidation state and sample temperature (25–450 °C) on the interaction with hydrogen. Our findings reveal that the oxidation state during hydrogen interaction involves a complex interplay between oxidizing hydride formation, reducing thermal reduction, and reducing formation of hydroxyls followed by water desorption. In all studied conditions, the subsurface exhibits a higher degree of oxidation compared to the surface, with a more subtle difference for the reduced sample. The reduced samples are significantly hydroxylated and covered with molecular water at 25 °C. We also investigate the impact of water vapor impurities in hydrogen. We find that although 1 × 10 –6 Torr water vapor oxidizes ceria, it is probably not the primary driver behind the oxidation of reduced ceria in the presence of hydrogen.

Topics & Concepts

HydrogenOxidation stateOxidizing agentX-ray photoelectron spectroscopyOxideInorganic chemistryThermal oxidationThin filmChemistryRedoxCeriumHydrideTorrCrystalliteWater vaporThermal desorptionCerium oxideDesorptionMaterials scienceMetalChemical engineeringAdsorptionPhysical chemistryCrystallographyNanotechnologyOrganic chemistryThermodynamicsPhysicsEngineeringCatalytic Processes in Materials ScienceElectronic and Structural Properties of OxidesRadioactive element chemistry and processing